Prof. François Légaré Profile

Prof. François Légaré

at Institut National de la Recherche Scientifique

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Author

Publications (4)

Proceedings Article | 13 March 2024 Presentation

250 kHz repetition rate OPA and 6 EV line for TR-ARPES measurement

Gaëtan Jargot, Adrien Longa, Jean-Michel Parent, Dario Armanno, Benson Frimpong, François Légaré, Fabio Boschini

Proceedings Volume PC12869, PC128690R (2024) https://doi.org/10.1117/12.3001015

KEYWORDS: Optical parametric amplifiers, Mid-IR, Difference frequency generation, Photoemission spectroscopy, Ultraviolet radiation, Ultrafast phenomena, Terahertz radiation, Quantum switching, Quantum probes, Quantum light generation

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Proceedings Article | 15 March 2023 Presentation + Paper

Imaging and controlling ultrafast dissociation dynamics: from conventional to surprising paths

Tomoyuki Endo, Simon Neville, Philippe Lassonde, Chen Qu, Bruno Schmidt, Mizuho Fushitani, Akiyoshi Hishikawa, Paul Houston, Joel Bowman, Michael Schuurman, François Légaré, Heide Ibrahim

Proceedings Volume 12419, 1241906 (2023) https://doi.org/10.1117/12.2649247

KEYWORDS: Molecules, Ultrafast imaging, Quantum processes, Quantum experiments, Ultrafast phenomena, Simulations, Chemistry, Vibration, Molecular lasers, Time resolved spectroscopy

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Proceedings Article | 30 May 2022 Presentation

Multimodal hollow-core fibers: a new route for few-cycle visible pulse generation

Riccardo Piccoli, Jeffrey Brown, Young-Gyun Jeong, Andrea Rovere, Luca Zanotto, Mette Gaarde, Francois Légaré, Arnaud Couairon, John Travers, Roberto Morandotti, Bruno Schmidt, Luca Razzari

Proceedings Volume PC12142, PC121420T (2022) https://doi.org/10.1117/12.2624288

KEYWORDS: Optical fibers, Visible radiation, Scanning probe microscopy, Pulsed laser operation, Plasma, Kerr effect, Energy transfer, Ultrafast phenomena, Transient nonlinear optics, Solids

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Ultrashort high-energy visible pulses have enabled unprecedented opportunities in temporally resolving ultrafast dynamics in physics, chemistry, and biology. Until now, high-energy sub-10 fs visible pulses have been mostly obtained through complex non-collinear optical parametric amplification setups, followed by some pulse post-compression technique. Here, we present an alternative approach, which relies on considering the typically-undesired multimode nature of large-core hollow-core capillary fibers (HCFs) as an essential asset. In our experiments, 1 mJ 175-fs-long pulses centered at 1035 nm, emitted by an Yb:KGW (Pharos – Light Conversion) laser, were coupled into a 3-m-long HCF (few-cycle Inc.) filled with Argon gas. At a selected pressure of 2.9 bar, a fast energy transfer from the laser broadened via self-phase modulation towards the arising visible light was observed starting at around 0.8 mJ laser pulse energy. At the maximum pulse energy of 0.94 mJ, a continuous spectrum of visible light between 800 nm and 400 nm was measured, with an overall energy of approximately 30 µJ. To understand this process, we implemented 3D carrier-resolved pulse propagation simulations based on the guided mode theory. The simulations predict the direct formation of a pulse of about 5 fs right at the exit of the fiber, considering the visible spectrum in the range 525 - 750 nm. We found that the presence of higher-order modes is crucial to generate such visible pulses and that the Kerr effect is the dominant nonlinearity enabling the modal energy transfer. Experimentally, we characterized the visible pulses by means of a transient-grating frequency-resolved optical gating setup (TG-FROG). At 0.94 mJ and 2.9 bar, a visible pulse duration of 4.6 fs was measured. We also implemented a cross-correlation TG-XFROG, using the separately-compressed laser light and the visible pulses, which demonstrates the possibility of directly implementing high-energy NIR-pump VIS-probe measurements on a sub-10-fs scale.

Proceedings Article | 5 March 2022 Presentation + Paper

Compressed ultrafast tomographic imaging using standard streak cameras

Yingming Lai, Ruibo Shang, Christian-Yves Côté, Xianglei Liu, Antoine Laramée, Francois Légaré, Geoffrey Luke, Jinyang Liang

Proceedings Volume 12008, 120080S (2022) https://doi.org/10.1117/12.2608938

KEYWORDS: Streak cameras, Ultrafast imaging, Tomography, Reconstruction algorithms, Cameras

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