Pulsed electron beam sources are increasingly in demand, especially as probes for ultrafast science and as patterning tools in lithography applications. Plasmonic nanostructures have been shown to enhance multiphoton photocurrent from metal cathodes by orders of magnitude, but for many applications it is also important to characterize the transverse electron beam properties. Here, we present preliminary work demonstrating a DC photogun setup for characterizing plasmonic photoemitters at Lawrence Berkeley National Laboratory, including measurement of photocurrent and the asymmetric transverse phase space of photoemitted beams from plasmonic nanogroove resonator arrays. This lays the groundwork for future studies of emerging plasmon-enhanced photoemitter designs, such as plasmonic lens nanoemitters.
Nanoscale electron pulses are increasingly in demand, including as probes of nanoscale ultrafast dynamics and for emerging light source and lithography applications. Using electromagnetic simulations, we show that gold plasmonic lenses as multiphoton photoemitters provide unique advantages, including emission from an atomically at surface, nanoscale pulse diameter regardless of laser spot size, and femtosecond-scale response time. We then present fabrication of prototypes with sub-nm roughness via e-beam lithography, as well as electro-optical characterization using cathodoluminescence spectromicroscopy. Finally, we introduce a DC photogun at LBNL built for testing ultrafast photoemitters. We discuss measurement considerations for ultrafast nanoemitters and predict that we can extract tens of pA photocurrent from a single plasmonic lens using a Ti:Sa oscillator. Altogether, this lays the groundwork to develop and test a broad class of plasmon-enhanced ultrafast nanoemitters.
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