Hyper Rayleigh and hyper Raman from neat water

Anthony Maurice; Qianli Ma; Isabelle Russier-Antoine; Emmanuel Benichou; Fabrice Canto; Laurent Couston; Pierre-François Brevet

doi:10.1117/12.2065133

27 August 2014 Hyper Rayleigh and hyper Raman from neat water

Anthony Maurice, Qianli Ma, Isabelle Russier-Antoine, Emmanuel Benichou, Fabrice Canto, Laurent Couston, Pierre-François Brevet

Author Affiliations +

Proceedings Volume 9171, Nanobiosystems: Processing, Characterization, and Applications VII; 91710S (2014) https://doi.org/10.1117/12.2065133
Event: SPIE NanoScience + Engineering, 2014, San Diego, California, United States

Abstract

Hyper Rayleigh and Hyper Raman spectra of neat water have been recorded in two different geometrical configurations where the incident fundamental beam is impinging on the cell at right angle from the collection direction and in retroreflection. A polarization analysis is also performed for the hyper Rayleigh experiment to underlines the differences in measuring some elements of the first hyperpolarizability tensor of the molecules present in the liquid solution under study. These data, beyond the comparison of the cross sections for the different bands observed, allows for a better insight into the quadratic nonlinear optical response from neat water.

Citation Download Citation

Anthony Maurice, Qianli Ma, Isabelle Russier-Antoine, Emmanuel Benichou, Fabrice Canto, Laurent Couston, and Pierre-François Brevet "Hyper Rayleigh and hyper Raman from neat water", Proc. SPIE 9171, Nanobiosystems: Processing, Characterization, and Applications VII, 91710S (27 August 2014); https://doi.org/10.1117/12.2065133

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