Theoretical description of SHG by fullerene film on dielectric surface

Mikhail M. Mestechkin; Gene Whyman

doi:10.1117/12.504614

10 November 2003 Theoretical description of SHG by fullerene film on dielectric surface

Mikhail M. Mestechkin, Gene Whyman

Proceedings Volume 5212, Linear and Nonlinear Optics of Organic Materials III; (2003) https://doi.org/10.1117/12.504614
Event: Optical Science and Technology, SPIE's 48th Annual Meeting, 2003, San Diego, California, United States

Abstract

The first hyperpolarizability (HP) of ullerene on the silica substructure, modeled by β-quartz layers, is calculated in the framework of the semi-empirical version of the time-dependent Hartree-Fock theory. The induced by the substrate orthogonal to the surface component of β-vector invariant is of the same order as in the 'push-pull' organic molecules with the expressed nonlinear optical properties. Just this component is responsible for generation of the second harmonic according to Hoshi and coauthors.

Citation Download Citation

Mikhail M. Mestechkin and Gene Whyman "Theoretical description of SHG by fullerene film on dielectric surface", Proc. SPIE 5212, Linear and Nonlinear Optics of Organic Materials III, (10 November 2003); https://doi.org/10.1117/12.504614

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