Open Access Presentation + Paper
20 September 2018 Spin-orbit coupling in vortex light: can it be revealed in fundamental electronic transitions?
Author Affiliations +
Abstract
Recent theoretical work on circular dichroic effects, for absorption processes in chiral materials, has reopened questions over the possibility that the interactions of vortex beams may display a sensitivity to material handedness. The interest in such a phenomenon arises from the fact that any engagement of optical phase gradients, in quadrupole-allowed electronic transitions, will represent a distinctive form of engagement with chiral matter. This is an issue that numerous careful experiments have so far failed to fully resolve, with some of them giving a clear null result, yet others giving positive indications. A definitive outcome from any such investigation would represent a touchstone for a broader, yet more challenging question: is there any mechanism by means of which twisted light, which conveys both orbital and spin angular momentum, can exhibit coupling between the two? It emerges that such a possibility can be identified, but the constraints upon its manifestation are severe. This presentation sets out the principles and the conclusions to which they lead, informing the pathway for ongoing experimentation.
Conference Presentation
© (2018) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Kayn A. Forbes and David L. Andrews "Spin-orbit coupling in vortex light: can it be revealed in fundamental electronic transitions?", Proc. SPIE 10732, Spintronics XI, 1073216 (20 September 2018); https://doi.org/10.1117/12.2320985
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KEYWORDS
Molecules

Dichroic materials

Absorption

Polarization

Structured light

Optical vortices

Light scattering

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