Presentation
15 March 2023 Formation of moiré interlayer excitons in space and time
Stefan Mathias
Author Affiliations +
Abstract
In my talk, I will present the ultrafast formation dynamics of dark interlayer excitons in twisted WSe2/MoS2 heterostructures in space and time. First, I will report on the identification of a hallmark signature of the moiré superlattice that is imprinted onto the momentum-resolved interlayer exciton photoemission signal. With this data, we reconstruct the electronic part of the exciton wavefunction, and relate its extension to the moiré wavelength of the heterostructure. Second, I will show that interlayer excitons are effectively formed via exciton-phonon scattering, and subsequent interlayer tunneling at the interlayer hybridized ΣW valleys on the sub-50 fs timescale.
Conference Presentation
© (2023) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Stefan Mathias "Formation of moiré interlayer excitons in space and time", Proc. SPIE PC12419, Ultrafast Phenomena and Nanophotonics XXVII, (15 March 2023); https://doi.org/10.1117/12.2651561
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KEYWORDS
Excitons

Heterojunctions

Quasiparticles

Ultrafast phenomena

Crystals

Microscopy

Scattering

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